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Frustration-induced one-dimensionality in the isosceles triangular antiferromagnetic lattice of δ-(EDT-TTF-CONMe2)2AsF6

Abstract : The 1/4-filled organic compound, δ-(EDT-TTF-CONMe2)2AsF6 is a frustrated two-dimensional triangular magnetic system as shown by high-frequency (111.2 and 222.4 GHz) electron spin resonance (ESR) and structural data in the literature. The material gradually orders antiferromagnetically below 40 K, but some magnetically disordered domains persist down to 4 K. We propose that in defect free regions frustration prevents true magnetic order down to at least 4 K in spite of the large first- and second-neighbor exchange interactions along chains and between chains, respectively. The antiferromagnetic (AFM) order gradually developing below 40 K nucleates around structural defects that locally cancel frustration. Two antiferromagnetic resonance modes mapped in the principal planes at 4 K are assigned to the very weakly interacting one-dimensional molecular chains in antiferromagnetic regions.
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Soumis le : mardi 5 mai 2020 - 17:38:36
Dernière modification le : jeudi 23 juillet 2020 - 09:42:05

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Bálint Náfrádi, Ágnes Antal, Titusz Fehér, Laszlo Kiss, Cécile Mézière, et al.. Frustration-induced one-dimensionality in the isosceles triangular antiferromagnetic lattice of δ-(EDT-TTF-CONMe2)2AsF6. Physical Review B, American Physical Society, 2016, 94 (17), pp.174413. ⟨10.1103/PhysRevB.94.174413⟩. ⟨hal-02564186⟩

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