Infrared spectra of the one-dimensional quarter-filled Wigner lattice compounds delta-(EDT-TTF-CONMe2)(2)X (X = AsF6, Br): Domain-wall excitations - Université d'Angers Accéder directement au contenu
Article Dans Une Revue Physical Review B: Condensed Matter and Materials Physics (1998-2015) Année : 2013

Infrared spectra of the one-dimensional quarter-filled Wigner lattice compounds delta-(EDT-TTF-CONMe2)(2)X (X = AsF6, Br): Domain-wall excitations

Ágnes Antal
  • Fonction : Auteur
T. Knoblauch
  • Fonction : Auteur
Martin Dressel
  • Fonction : Auteur
Patrick Batail
  • Fonction : Auteur
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Natalia Drichko
  • Fonction : Auteur

Résumé

Optical investigations of quarter-filled charge ordered insulators delta-(EDT-TTF-CONMe2)(2)X, X = AsF6, Br are reported. The spectra evidence the one-dimensional nature of the systems at all temperatures. The charge order exists already at room temperature, the optical gap is estimated to be of the order of 550 cm(-1) for the X = Br compound and about 700 cm(-1) for the X = AsF6 material. The optical response in the direction of the stacks is discussed in terms of domain-wall excitations of one-dimensional quarter-filled Wigner lattice at moderate values of nearest-neighbor electronic repulsion. A similarity between the effects of temperature contraction and chemical pressure is found.

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Chimie
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Dates et versions

hal-03344531 , version 1 (15-09-2021)

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Ágnes Antal, T. Knoblauch, Martin Dressel, Patrick Batail, Natalia Drichko. Infrared spectra of the one-dimensional quarter-filled Wigner lattice compounds delta-(EDT-TTF-CONMe2)(2)X (X = AsF6, Br): Domain-wall excitations. Physical Review B: Condensed Matter and Materials Physics (1998-2015), 2013, 87 (7), Non spécifié. ⟨10.1103/PhysRevB.87.075118⟩. ⟨hal-03344531⟩
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